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Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films

Hui Liu, Hairui Liu, Jien Yang, Feng Yang, Zhiyong Liu, Sagar Jain

Crystal Growth & Design

Swansea University Author: Sagar Jain

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DOI (Published version): 10.1021/acs.cgd.9b00024

Abstract

Obtaining good quality perovskite absorber film remains a challenging task that limits performance of planar perovskite solar cells. . In this work, we demonstrated the importance of pre-heating treatment on perovskite nucleation and phase transition. . Fine-tuning the appropriate pre-heating and st...

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Published in: Crystal Growth & Design
ISSN: 1528-7483 1528-7505
Published: 2019
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URI: https://cronfa.swan.ac.uk/Record/cronfa50828
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spelling 2019-06-14T15:59:51.7430184 v2 50828 2019-06-14 Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films 7073e179bb5b82db3e3efd3a8cd07139 Sagar Jain Sagar Jain true false 2019-06-14 EEN Obtaining good quality perovskite absorber film remains a challenging task that limits performance of planar perovskite solar cells. . In this work, we demonstrated the importance of pre-heating treatment on perovskite nucleation and phase transition. . Fine-tuning the appropriate pre-heating and standing time resulted in the formation of high quality perovskite films with enhanced optoelectronic properties.. Pre-heated perovskite films with delaying of 1 hour post-annealing achieved the hysteresis-free, record power conversion efficiency (PCE) of 16.18%. While the perovskite films without preheating treatment in solar cells shown only12.35% efficiency.. This improved performance with pre-heating treatment and delay annealing of perovskite films found as a result of homogeneous nucleation and formation of high quality perovskite films. Improved perovskite quality is further evidenced from enhanced optoelectronic and crystalline properties of the perovskite absorber after preheating treatment. Journal Article Crystal Growth & Design 1528-7483 1528-7505 10 6 2019 2019-06-10 10.1021/acs.cgd.9b00024 COLLEGE NANME Engineering COLLEGE CODE EEN Swansea University 2019-06-14T15:59:51.7430184 2019-06-14T15:57:27.0878862 Faculty of Science and Engineering School of Engineering and Applied Sciences - Uncategorised Hui Liu 1 Hairui Liu 2 Jien Yang 3 Feng Yang 4 Zhiyong Liu 5 Sagar Jain 6 0050828-14062019155934.pdf liu2019v2.pdf 2019-06-14T15:59:34.8200000 Output 9996162 application/pdf Accepted Manuscript true 2020-06-10T00:00:00.0000000 false eng
title Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films
spellingShingle Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films
Sagar Jain
title_short Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films
title_full Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films
title_fullStr Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films
title_full_unstemmed Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films
title_sort Improving the Performance of Planar Perovskite Solar Cells through Pre-heated, Delaying Annealing Process to Control Nucleation and Phase Transition of Perovskite Films
author_id_str_mv 7073e179bb5b82db3e3efd3a8cd07139
author_id_fullname_str_mv 7073e179bb5b82db3e3efd3a8cd07139_***_Sagar Jain
author Sagar Jain
author2 Hui Liu
Hairui Liu
Jien Yang
Feng Yang
Zhiyong Liu
Sagar Jain
format Journal article
container_title Crystal Growth & Design
publishDate 2019
institution Swansea University
issn 1528-7483
1528-7505
doi_str_mv 10.1021/acs.cgd.9b00024
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Uncategorised{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Uncategorised
document_store_str 1
active_str 0
description Obtaining good quality perovskite absorber film remains a challenging task that limits performance of planar perovskite solar cells. . In this work, we demonstrated the importance of pre-heating treatment on perovskite nucleation and phase transition. . Fine-tuning the appropriate pre-heating and standing time resulted in the formation of high quality perovskite films with enhanced optoelectronic properties.. Pre-heated perovskite films with delaying of 1 hour post-annealing achieved the hysteresis-free, record power conversion efficiency (PCE) of 16.18%. While the perovskite films without preheating treatment in solar cells shown only12.35% efficiency.. This improved performance with pre-heating treatment and delay annealing of perovskite films found as a result of homogeneous nucleation and formation of high quality perovskite films. Improved perovskite quality is further evidenced from enhanced optoelectronic and crystalline properties of the perovskite absorber after preheating treatment.
published_date 2019-06-10T04:02:27Z
_version_ 1763753221150474240
score 10.999547

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