Practical challenges in the development of photoelectrochemical solar fuels production

Spitler, Mark T.; Modestino, Miguel A.; Deutsch, Todd G.; Xiang, Chengxiang X.; Durrant, James; Esposito, Daniel V.; Haussener, Sophia; Maldonado, Stephen; Sharp, Ian D.; Parkinson, Bruce A.; Ginley, David S.; Houle, Frances A.; Hannappel, Thomas; Neale, Nathan R.; Nocera, Daniel G.; McIntyre, Paul C.

doi:10.1039/c9se00869a

Journal article 375 views

Practical challenges in the development of photoelectrochemical solar fuels production

Mark T. Spitler, Miguel A. Modestino, Todd G. Deutsch, Chengxiang X. Xiang, James Durrant

, Daniel V. Esposito, Sophia Haussener, Stephen Maldonado, Ian D. Sharp, Bruce A. Parkinson, David S. Ginley, Frances A. Houle, Thomas Hannappel, Nathan R. Neale, Daniel G. Nocera, Paul C. McIntyre

Sustainable Energy & Fuels, Volume: 4, Issue: 3, Pages: 985 - 995

Swansea University Author: James Durrant

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DOI (Published version): 10.1039/c9se00869a

Abstract

This article addresses the challenges presented by photoelectrochemical solar fuels technology in a discussion that begins with a functioning device and proceeds to the more fundamental science of its component parts. In this flow of discussion issues are addressed that frame the discussion for the...

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Published in:	Sustainable Energy & Fuels
ISSN:	2398-4902
Published:	Royal Society of Chemistry (RSC) 2020
Online Access:	Check full text
URI:	https://cronfa.swan.ac.uk/Record/cronfa53835
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first_indexed	2020-03-19T13:53:08Z
last_indexed	2020-09-17T03:17:17Z
id	cronfa53835
recordtype	SURis
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spelling	2020-03-19T10:45:24.5799624 v2 53835 2020-03-19 Practical challenges in the development of photoelectrochemical solar fuels production f3dd64bc260e5c07adfa916c27dbd58a 0000-0001-8353-7345 James Durrant James Durrant true false 2020-03-19 MTLS This article addresses the challenges presented by photoelectrochemical solar fuels technology in a discussion that begins with a functioning device and proceeds to the more fundamental science of its component parts. In this flow of discussion issues are addressed that frame the discussion for the next, increasingly more fundamental topic. The analysis begins with a discussion of the need for an analytical facility for confirmation of reported efficiencies of solar fuels device prototypes and then progressively narrows its scope to prototype design, the discovery of novel materials and the design of durable interfacial structures for fuels evolution. Molecular hydrogen will be considered first as the target fuel since many of the challenges with hydrogen production are general and applicable to the more complex CO2 reduction, which will be treated as a supplementary subject. Journal Article Sustainable Energy & Fuels 4 3 985 995 Royal Society of Chemistry (RSC) 2398-4902 1 3 2020 2020-03-01 10.1039/c9se00869a COLLEGE NANME Materials Science and Engineering COLLEGE CODE MTLS Swansea University 2020-03-19T10:45:24.5799624 2020-03-19T10:45:24.5799624 Mark T. Spitler 1 Miguel A. Modestino 2 Todd G. Deutsch 3 Chengxiang X. Xiang 4 James Durrant 0000-0001-8353-7345 5 Daniel V. Esposito 6 Sophia Haussener 7 Stephen Maldonado 8 Ian D. Sharp 9 Bruce A. Parkinson 10 David S. Ginley 11 Frances A. Houle 12 Thomas Hannappel 13 Nathan R. Neale 14 Daniel G. Nocera 15 Paul C. McIntyre 16
title	Practical challenges in the development of photoelectrochemical solar fuels production
spellingShingle	Practical challenges in the development of photoelectrochemical solar fuels production James Durrant
title_short	Practical challenges in the development of photoelectrochemical solar fuels production
title_full	Practical challenges in the development of photoelectrochemical solar fuels production
title_fullStr	Practical challenges in the development of photoelectrochemical solar fuels production
title_full_unstemmed	Practical challenges in the development of photoelectrochemical solar fuels production
title_sort	Practical challenges in the development of photoelectrochemical solar fuels production
author_id_str_mv	f3dd64bc260e5c07adfa916c27dbd58a
author_id_fullname_str_mv	f3dd64bc260e5c07adfa916c27dbd58a_***_James Durrant
author	James Durrant
author2	Mark T. Spitler Miguel A. Modestino Todd G. Deutsch Chengxiang X. Xiang James Durrant Daniel V. Esposito Sophia Haussener Stephen Maldonado Ian D. Sharp Bruce A. Parkinson David S. Ginley Frances A. Houle Thomas Hannappel Nathan R. Neale Daniel G. Nocera Paul C. McIntyre
format	Journal article
container_title	Sustainable Energy & Fuels
container_volume	4
container_issue	3
container_start_page	985
publishDate	2020
institution	Swansea University
issn	2398-4902
doi_str_mv	10.1039/c9se00869a
publisher	Royal Society of Chemistry (RSC)
document_store_str	0
active_str	0
description	This article addresses the challenges presented by photoelectrochemical solar fuels technology in a discussion that begins with a functioning device and proceeds to the more fundamental science of its component parts. In this flow of discussion issues are addressed that frame the discussion for the next, increasingly more fundamental topic. The analysis begins with a discussion of the need for an analytical facility for confirmation of reported efficiencies of solar fuels device prototypes and then progressively narrows its scope to prototype design, the discovery of novel materials and the design of durable interfacial structures for fuels evolution. Molecular hydrogen will be considered first as the target fuel since many of the challenges with hydrogen production are general and applicable to the more complex CO2 reduction, which will be treated as a supplementary subject.
published_date	2020-03-01T04:07:00Z
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score	11.012678

Practical challenges in the development of photoelectrochemical solar fuels production

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