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The application of amine-based materials for carbon capture and utilisation: an overarching view

Louise Hamdy, Chitrakshi Goel, Jennifer Rudd Orcid Logo, Andrew Barron Orcid Logo, Enrico Andreoli Orcid Logo

Materials Advances, Volume: 2, Issue: 18, Pages: 5843 - 5880

Swansea University Authors: Louise Hamdy, Chitrakshi Goel, Jennifer Rudd Orcid Logo, Andrew Barron Orcid Logo, Enrico Andreoli Orcid Logo

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DOI (Published version): 10.1039/d1ma00360g

Abstract

In the ongoing research campaign to reduce the global atmospheric CO2 concentration, technologies are being developed to enable the capture of CO2 from dilute sources and conversion into higher-value products. Amine and polyamine-based materials feature widely in the literature as solid CO2 sorbents...

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Published in: Materials Advances
ISSN: 2633-5409
Published: Royal Society of Chemistry (RSC) 2021
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URI: https://cronfa.swan.ac.uk/Record/cronfa57952
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Amine and polyamine-based materials feature widely in the literature as solid CO2 sorbents and as catalyst modifiers for CO2 electrochemical reduction; however, advancing lab-scale research into a pilot or industrial-scale application is fraught with challenges, starting with the definition and identification of an effective adsorbent. This multidisciplinary review serves as an essential introduction to the role of amines in carbon capture and utilisation for scientists entering and advancing the field. The chemical and engineering principles of amine-based CO2 capture are considered to define the parameters required of an adsorbent, describe adsorption testing methods, and introduce the reader to a range of amine-based adsorbents and how they can be specialised to overcome specific issues. 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spelling 2021-10-18T13:19:23.4243088 v2 57952 2021-09-18 The application of amine-based materials for carbon capture and utilisation: an overarching view 7f3a162e82c925cadead8a3b8d37dc81 Louise Hamdy Louise Hamdy true false 85b5d4216725a712415370decc448186 Chitrakshi Goel Chitrakshi Goel true false c2e4cf0f048a86b5ca2f331e6c566aff 0000-0002-5209-477X Jennifer Rudd Jennifer Rudd true false 92e452f20936d688d36f91c78574241d 0000-0002-2018-8288 Andrew Barron Andrew Barron true false cbd843daab780bb55698a3daccd74df8 0000-0002-1207-2314 Enrico Andreoli Enrico Andreoli true false 2021-09-18 EEN In the ongoing research campaign to reduce the global atmospheric CO2 concentration, technologies are being developed to enable the capture of CO2 from dilute sources and conversion into higher-value products. Amine and polyamine-based materials feature widely in the literature as solid CO2 sorbents and as catalyst modifiers for CO2 electrochemical reduction; however, advancing lab-scale research into a pilot or industrial-scale application is fraught with challenges, starting with the definition and identification of an effective adsorbent. This multidisciplinary review serves as an essential introduction to the role of amines in carbon capture and utilisation for scientists entering and advancing the field. The chemical and engineering principles of amine-based CO2 capture are considered to define the parameters required of an adsorbent, describe adsorption testing methods, and introduce the reader to a range of amine-based adsorbents and how they can be specialised to overcome specific issues. Finally, the application of electrocatalysts modified with nitrogen-containing compounds and polymers is reviewed in the context of CO2 utilisation. Journal Article Materials Advances 2 18 5843 5880 Royal Society of Chemistry (RSC) 2633-5409 1 9 2021 2021-09-01 10.1039/d1ma00360g COLLEGE NANME Engineering COLLEGE CODE EEN Swansea University Reducing Industrial Carbon Emissions (RICE) and Flexible Integrated Energy Systems (FLEXIS) research operations part-funded by the EU’s European Regional Development Fund through the Welsh Government. Support was also provided by the Engineering and Physical Sciences Research Council through the SUSTAIN Manufacturing Hub EP/S018107/1 and project EP/N009525/1. 2021-10-18T13:19:23.4243088 2021-09-18T07:11:50.5768633 Faculty of Science and Engineering School of Engineering and Applied Sciences - Chemical Engineering Louise Hamdy 1 Chitrakshi Goel 2 Jennifer Rudd 0000-0002-5209-477X 3 Andrew Barron 0000-0002-2018-8288 4 Enrico Andreoli 0000-0002-1207-2314 5 57952__21082__6110570ddebb41bd8851d94af78e4e06.pdf 57952.pdf 2021-10-04T12:31:09.8597343 Output 7610472 application/pdf Version of Record true © 2021 The Author(s). This article is licensed under a Creative Commons Attribution 3.0 Unported Licence true eng http://creativecommons.org/licenses/by/3.0/
title The application of amine-based materials for carbon capture and utilisation: an overarching view
spellingShingle The application of amine-based materials for carbon capture and utilisation: an overarching view
Louise Hamdy
Chitrakshi Goel
Jennifer Rudd
Andrew Barron
Enrico Andreoli
title_short The application of amine-based materials for carbon capture and utilisation: an overarching view
title_full The application of amine-based materials for carbon capture and utilisation: an overarching view
title_fullStr The application of amine-based materials for carbon capture and utilisation: an overarching view
title_full_unstemmed The application of amine-based materials for carbon capture and utilisation: an overarching view
title_sort The application of amine-based materials for carbon capture and utilisation: an overarching view
author_id_str_mv 7f3a162e82c925cadead8a3b8d37dc81
85b5d4216725a712415370decc448186
c2e4cf0f048a86b5ca2f331e6c566aff
92e452f20936d688d36f91c78574241d
cbd843daab780bb55698a3daccd74df8
author_id_fullname_str_mv 7f3a162e82c925cadead8a3b8d37dc81_***_Louise Hamdy
85b5d4216725a712415370decc448186_***_Chitrakshi Goel
c2e4cf0f048a86b5ca2f331e6c566aff_***_Jennifer Rudd
92e452f20936d688d36f91c78574241d_***_Andrew Barron
cbd843daab780bb55698a3daccd74df8_***_Enrico Andreoli
author Louise Hamdy
Chitrakshi Goel
Jennifer Rudd
Andrew Barron
Enrico Andreoli
author2 Louise Hamdy
Chitrakshi Goel
Jennifer Rudd
Andrew Barron
Enrico Andreoli
format Journal article
container_title Materials Advances
container_volume 2
container_issue 18
container_start_page 5843
publishDate 2021
institution Swansea University
issn 2633-5409
doi_str_mv 10.1039/d1ma00360g
publisher Royal Society of Chemistry (RSC)
college_str Faculty of Science and Engineering
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hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Chemical Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Chemical Engineering
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description In the ongoing research campaign to reduce the global atmospheric CO2 concentration, technologies are being developed to enable the capture of CO2 from dilute sources and conversion into higher-value products. Amine and polyamine-based materials feature widely in the literature as solid CO2 sorbents and as catalyst modifiers for CO2 electrochemical reduction; however, advancing lab-scale research into a pilot or industrial-scale application is fraught with challenges, starting with the definition and identification of an effective adsorbent. This multidisciplinary review serves as an essential introduction to the role of amines in carbon capture and utilisation for scientists entering and advancing the field. The chemical and engineering principles of amine-based CO2 capture are considered to define the parameters required of an adsorbent, describe adsorption testing methods, and introduce the reader to a range of amine-based adsorbents and how they can be specialised to overcome specific issues. Finally, the application of electrocatalysts modified with nitrogen-containing compounds and polymers is reviewed in the context of CO2 utilisation.
published_date 2021-09-01T04:14:05Z
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score 10.998093

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