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Identification and Prioritisation of Mine Pollution Sources in a Temperate Watershed Using Tracer Injection and Synoptic Sampling

Patrick Byrne, Alan Yendell, Ilaria Frau, Brown Todd Orcid Logo

Mine Water and the Environment, Volume: 40, Issue: 4, Pages: 980 - 993

Swansea University Author: Brown Todd Orcid Logo

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Abstract

Identifying and prioritising mine sites for remediation is challenging due to inherently complex hydrological systems and multiple potential sources of mine pollution dispersed across watersheds. Understanding mine pollution dynamics in wet temperate watersheds is particularly challenging due to sub...

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Published in: Mine Water and the Environment
ISSN: 1025-9112 1616-1068
Published: Springer Science and Business Media LLC 2021
Online Access: Check full text

URI: https://cronfa.swan.ac.uk/Record/cronfa58374
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Abstract: Identifying and prioritising mine sites for remediation is challenging due to inherently complex hydrological systems and multiple potential sources of mine pollution dispersed across watersheds. Understanding mine pollution dynamics in wet temperate watersheds is particularly challenging due to substantial variability in precipitation and streamflows, which increase the importance of diffuse sources. A tracer dilution and synoptic sampling experiment was conducted in a mined watershed in Scotland to identify the main sources of mine pollution, the relative importance of point and diffuse sources of pollution, and the potential benefits of mine site remediation to stream water quality. Using high spatial resolution metal loading datasets, the major Zn and Cd source areas were identified as point sources of mine water predominantly located in the upper part of the watershed. In contrast, the main sources of Pb were diffuse sources of mine tailings and wastes located in the lower part of the watershed. In the latter case, mobilisation of Pb occurred primarily from a section of braided wetland and an uncapped tailings area. Importantly, diffuse sources of mine pollution were found to be the dominant source of Pb, and an important source of Zn and Cd, even under steady-state streamflow conditions. Mass balance calculations suggest that treatment of the main mine water sources in the upper watershed and capping of the tailings deposit in the lower watershed could reduce stream trace metal concentrations by approximately 70%. These data support the development of conceptual models of mine pollution dynamics in wet temperate watersheds. These conceptual models are important as they: (1) help prioritise those mine sites and features for remediation that will deliver the most environmental and socio-economic benefit, and; (2) provide a means to quantify the importance of diffuse pollution sources that may increase in importance in the future as a result of changes in precipitation patterns in temperate watersheds.
Keywords: Mining; Metal; Scotland; Water quality; Difuse pollution; Remediation
College: Faculty of Science and Engineering
Funders: This project was supported by the SEPA Research and Development fund as part of its R&D work for novel water monitoring techniques to support identification of pollutant sources.
Issue: 4
Start Page: 980
End Page: 993