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Downconversion Materials for Perovskite Solar Cells

Ram Datt, Swati Bishnoi, Declan Hughes Orcid Logo, Prerna Mahajan, Anoop Singh, Ramashanker Gupta, Sandeep Arya, Vinay Gupta, Wing Chung Tsoi Orcid Logo

Solar RRL, Volume: 6, Issue: 8, Start page: 2200266

Swansea University Authors: Ram Datt, Declan Hughes Orcid Logo, Wing Chung Tsoi Orcid Logo

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DOI (Published version): 10.1002/solr.202200266

Abstract

Perovskite solar cells (PSCs) have made game changing progress during the last decade and reached a power conversion efficiency (PCE) of up to 25%. Furthermore, the development of material chemistry, structure design, active layer composition, and process engineering, etc. have contributed to improv...

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Published in: Solar RRL
ISSN: 2367-198X 2367-198X
Published: Wiley 2022
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URI: https://cronfa.swan.ac.uk/Record/cronfa60054
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Furthermore, the development of material chemistry, structure design, active layer composition, and process engineering, etc. have contributed to improving PSCs stability. The significant PCE losses experienced by PSCs are related to spectral mismatch between the incident solar spectra and absorption range of active layer, which thereby limits the PCE. Besides PSCs performance, the photoinduced degradation is also a major concern. Recently, lanthanide (rare-earth) and non-lanthanide based down-conversion (DC) materials have been introduced to resolve these spectral mismatch losses as well as to reduce the photoinduced degradation. The DC materials improve the photovoltaic performance by converting ultraviolet (UV) light to visible, also providing UV shielding, and thus contribute to increasing the efficiency as well as stability of the PSCs. Moreover, the Shockley-Queisser efficiency limit of the solar cell could be crossed with the help of DC materials. 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spelling 2022-08-31T12:10:43.7661778 v2 60054 2022-05-19 Downconversion Materials for Perovskite Solar Cells 350d1f64ddd9787a6eda98611dcbb8d2 Ram Datt Ram Datt true false 5590b62d833b89a43926267b2b7a5c29 0000-0001-6415-3717 Declan Hughes Declan Hughes true false 7e5f541df6635a9a8e1a579ff2de5d56 0000-0003-3836-5139 Wing Chung Tsoi Wing Chung Tsoi true false 2022-05-19 MTLS Perovskite solar cells (PSCs) have made game changing progress during the last decade and reached a power conversion efficiency (PCE) of up to 25%. Furthermore, the development of material chemistry, structure design, active layer composition, and process engineering, etc. have contributed to improving PSCs stability. The significant PCE losses experienced by PSCs are related to spectral mismatch between the incident solar spectra and absorption range of active layer, which thereby limits the PCE. Besides PSCs performance, the photoinduced degradation is also a major concern. Recently, lanthanide (rare-earth) and non-lanthanide based down-conversion (DC) materials have been introduced to resolve these spectral mismatch losses as well as to reduce the photoinduced degradation. The DC materials improve the photovoltaic performance by converting ultraviolet (UV) light to visible, also providing UV shielding, and thus contribute to increasing the efficiency as well as stability of the PSCs. Moreover, the Shockley-Queisser efficiency limit of the solar cell could be crossed with the help of DC materials. In this review, we have thoroughly discussed the importance, processing, and the reported DC materials for PSCs. Furthermore, the development of DC materials and their impact on PSCs performance and stability, along with their future perspectives has been focused. Journal Article Solar RRL 6 8 2200266 Wiley 2367-198X 2367-198X down-conversion; lanthanides; non-lanthanides; perovskite solar cells; stability 1 8 2022 2022-08-01 10.1002/solr.202200266 COLLEGE NANME Materials Science and Engineering COLLEGE CODE MTLS Swansea University SU Library paid the OA fee (TA Institutional Deal) UKRI, EPSRC (EP/N020863/1; EP/T028513/1) 2022-08-31T12:10:43.7661778 2022-05-19T17:19:24.8451267 Faculty of Science and Engineering School of Engineering and Applied Sciences - Materials Science and Engineering Ram Datt 1 Swati Bishnoi 2 Declan Hughes 0000-0001-6415-3717 3 Prerna Mahajan 4 Anoop Singh 5 Ramashanker Gupta 6 Sandeep Arya 7 Vinay Gupta 8 Wing Chung Tsoi 0000-0003-3836-5139 9 60054__24381__27697f22b16d45d08326a59c667136d6.pdf 60054.pdf 2022-06-23T13:49:18.9069716 Output 3700142 application/pdf Version of Record true © 2022 The Authors. This is an open access article under the terms of the Creative Commons Attribution License true eng http://creativecommons.org/licenses/by/4.0/
title Downconversion Materials for Perovskite Solar Cells
spellingShingle Downconversion Materials for Perovskite Solar Cells
Ram Datt
Declan Hughes
Wing Chung Tsoi
title_short Downconversion Materials for Perovskite Solar Cells
title_full Downconversion Materials for Perovskite Solar Cells
title_fullStr Downconversion Materials for Perovskite Solar Cells
title_full_unstemmed Downconversion Materials for Perovskite Solar Cells
title_sort Downconversion Materials for Perovskite Solar Cells
author_id_str_mv 350d1f64ddd9787a6eda98611dcbb8d2
5590b62d833b89a43926267b2b7a5c29
7e5f541df6635a9a8e1a579ff2de5d56
author_id_fullname_str_mv 350d1f64ddd9787a6eda98611dcbb8d2_***_Ram Datt
5590b62d833b89a43926267b2b7a5c29_***_Declan Hughes
7e5f541df6635a9a8e1a579ff2de5d56_***_Wing Chung Tsoi
author Ram Datt
Declan Hughes
Wing Chung Tsoi
author2 Ram Datt
Swati Bishnoi
Declan Hughes
Prerna Mahajan
Anoop Singh
Ramashanker Gupta
Sandeep Arya
Vinay Gupta
Wing Chung Tsoi
format Journal article
container_title Solar RRL
container_volume 6
container_issue 8
container_start_page 2200266
publishDate 2022
institution Swansea University
issn 2367-198X
2367-198X
doi_str_mv 10.1002/solr.202200266
publisher Wiley
college_str Faculty of Science and Engineering
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hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Materials Science and Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Materials Science and Engineering
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description Perovskite solar cells (PSCs) have made game changing progress during the last decade and reached a power conversion efficiency (PCE) of up to 25%. Furthermore, the development of material chemistry, structure design, active layer composition, and process engineering, etc. have contributed to improving PSCs stability. The significant PCE losses experienced by PSCs are related to spectral mismatch between the incident solar spectra and absorption range of active layer, which thereby limits the PCE. Besides PSCs performance, the photoinduced degradation is also a major concern. Recently, lanthanide (rare-earth) and non-lanthanide based down-conversion (DC) materials have been introduced to resolve these spectral mismatch losses as well as to reduce the photoinduced degradation. The DC materials improve the photovoltaic performance by converting ultraviolet (UV) light to visible, also providing UV shielding, and thus contribute to increasing the efficiency as well as stability of the PSCs. Moreover, the Shockley-Queisser efficiency limit of the solar cell could be crossed with the help of DC materials. In this review, we have thoroughly discussed the importance, processing, and the reported DC materials for PSCs. Furthermore, the development of DC materials and their impact on PSCs performance and stability, along with their future perspectives has been focused.
published_date 2022-08-01T04:17:50Z
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