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PEARS: A Web Tool for Fitting Time-Resolved Photoluminescence Decays of Perovskite Materials
Journal of Chemical Information and Modeling, Volume: 63, Issue: 15, Pages: 4477 - 4482
Swansea University Authors:
Emmanuel Pean, Matthew Davies
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DOI (Published version): 10.1021/acs.jcim.3c00217
Abstract
Time-resolved photoluminescence (TRPL) is a powerful tool to investigate charge carrier recombination processes in emissive materials. Perovskite materials are extremely promising for applications in solar cells; however, the interpretation of their TRPL is arduous due to the complicated nature of t...
| Published in: | Journal of Chemical Information and Modeling |
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| ISSN: | 1549-9596 1549-960X |
| Published: |
American Chemical Society (ACS)
2023
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| Online Access: |
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| URI: | https://cronfa.swan.ac.uk/Record/cronfa63951 |
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| Abstract: |
Time-resolved photoluminescence (TRPL) is a powerful tool to investigate charge carrier recombination processes in emissive materials. Perovskite materials are extremely promising for applications in solar cells; however, the interpretation of their TRPL is arduous due to the complicated nature of the recombination processes occurring in these materials. We present here the PErovskite cArrier Recombination Simulator (PEARS) web tool for effortlessly and quickly fitting TRPL of perovskite materials using advanced charge carrier recombination models, allowing for the extraction of recombination rate constants and trap state concentration. PEARS is flexible and can adapt to different situations, by ignoring recombination processes or fixing known parameters (e.g., the doping concentration). The tool is publicly available at https://pears-tool.herokuapp.com. |
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| Item Description: |
Application Note |
| Keywords: |
PEARS, time-resolved photoluminescence, TRPL, perovskite materials, solar cells |
| College: |
Faculty of Science and Engineering |
| Funders: |
We are grateful for the financial support of the EPSRC (EP/S001336/1, EP/R016666/1, and EP/N020863/1), Innovate UK (920036), and the European Regional Development Fund (c80892) through the Welsh Government for the SPECIFIC Innovation and Knowledge Centre. E.V.P. is grateful for funding through the IMPACT project. |
| Issue: |
15 |
| Start Page: |
4477 |
| End Page: |
4482 |