Journal article 7 views 3 downloads
Integrated CO2 capture and utilization with CaO-alone for high purity syngas production
Carbon Capture Science & Technology, Volume: 1, Start page: 100001
Swansea University Author:
Yuanting Qiao
-
PDF | Version of Record
© 2021 The Author(s). This is an open access article under the CC BY-NC-ND license.
Download (1.48MB)
DOI (Published version): 10.1016/j.ccst.2021.100001
Abstract
Carbon capture and utilization (CCU) represent a promising strategy to reduce CO2 emissions and promote a sustainable economy. We report an integrated CCU (ICCU) process by integrating CO2 capture with reverse water gas shift reaction by applying simple and low-cost CaO as both sorbent and catalyst....
Published in: | Carbon Capture Science & Technology |
---|---|
ISSN: | 2772-6568 |
Published: |
Elsevier BV
2021
|
Online Access: |
Check full text
|
URI: | https://cronfa.swan.ac.uk/Record/cronfa67100 |
Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
first_indexed |
2024-08-30T11:29:17Z |
---|---|
last_indexed |
2024-08-30T11:29:17Z |
id |
cronfa67100 |
recordtype |
SURis |
fullrecord |
<?xml version="1.0" encoding="utf-8"?><rfc1807 xmlns:xsi="http://www.w3.org/2001/XMLSchema-instance" xmlns:xsd="http://www.w3.org/2001/XMLSchema"><bib-version>v2</bib-version><id>67100</id><entry>2024-07-15</entry><title>Integrated CO2 capture and utilization with CaO-alone for high purity syngas production</title><swanseaauthors><author><sid>ceae57100ecb7c4b2883e29079a8985d</sid><ORCID>0000-0002-7741-9278</ORCID><firstname>Yuanting</firstname><surname>Qiao</surname><name>Yuanting Qiao</name><active>true</active><ethesisStudent>false</ethesisStudent></author></swanseaauthors><date>2024-07-15</date><deptcode>EAAS</deptcode><abstract>Carbon capture and utilization (CCU) represent a promising strategy to reduce CO2 emissions and promote a sustainable economy. We report an integrated CCU (ICCU) process by integrating CO2 capture with reverse water gas shift reaction by applying simple and low-cost CaO as both sorbent and catalyst. By switching the feeding gas from CO2 source to H2 isothermally, up to 75% of captured CO2 was 100% converted into CO at 600-700 °C and the cycle performance of CaO was significantly improved under ICCU condition. In addition, the simulation confirms the significant economic advantage compared to similar traditional processes. The work could dramatically reduce the cost of materials and simplify CCU processes to advance the development and deployment of carbon neutrality technologies.One-Sentence Summary: A low-cost and widely used material, CaO, was used to not only adsorb CO2 efficiently but also in situ convert CO2 into valuable syngas with > 75% CO2 conversion to realise carbon neutrality, which is a vital target for sustainable future development.</abstract><type>Journal Article</type><journal>Carbon Capture Science &amp; Technology</journal><volume>1</volume><journalNumber/><paginationStart>100001</paginationStart><paginationEnd/><publisher>Elsevier BV</publisher><placeOfPublication/><isbnPrint/><isbnElectronic/><issnPrint>2772-6568</issnPrint><issnElectronic/><keywords/><publishedDay>1</publishedDay><publishedMonth>12</publishedMonth><publishedYear>2021</publishedYear><publishedDate>2021-12-01</publishedDate><doi>10.1016/j.ccst.2021.100001</doi><url/><notes/><college>COLLEGE NANME</college><department>Engineering and Applied Sciences School</department><CollegeCode>COLLEGE CODE</CollegeCode><DepartmentCode>EAAS</DepartmentCode><institution>Swansea University</institution><apcterm/><funders>China Scholarship Council grant 201906450023
Marie Skłodowska-Curie grant No 823745</funders><projectreference/><lastEdited>2024-08-30T12:31:43.3001482</lastEdited><Created>2024-07-15T11:14:04.3273634</Created><path><level id="1">Faculty of Science and Engineering</level><level id="2">School of Engineering and Applied Sciences - Chemical Engineering</level></path><authors><author><firstname>Shuzhuang</firstname><surname>Sun</surname><order>1</order></author><author><firstname>Zongze</firstname><surname>Lv</surname><order>2</order></author><author><firstname>Yuanting</firstname><surname>Qiao</surname><orcid>0000-0002-7741-9278</orcid><order>3</order></author><author><firstname>Changlei</firstname><surname>Qin</surname><orcid>0000-0001-6744-4608</orcid><order>4</order></author><author><firstname>Shaojun</firstname><surname>Xu</surname><orcid>0000-0002-8026-8714</orcid><order>5</order></author><author><firstname>Chunfei</firstname><surname>Wu</surname><orcid>0000-0001-7961-1186</orcid><order>6</order></author></authors><documents><document><filename>67100__31184__9122651c24674c82a415fa0db0d812b0.pdf</filename><originalFilename>67100.VoR.pdf</originalFilename><uploaded>2024-08-30T12:29:58.2904816</uploaded><type>Output</type><contentLength>1549226</contentLength><contentType>application/pdf</contentType><version>Version of Record</version><cronfaStatus>true</cronfaStatus><documentNotes>© 2021 The Author(s). This is an open access article under the CC BY-NC-ND license.</documentNotes><copyrightCorrect>true</copyrightCorrect><language>eng</language><licence>http://creativecommons.org/licenses/by-nc-nd/4.0/</licence></document></documents><OutputDurs/></rfc1807> |
spelling |
v2 67100 2024-07-15 Integrated CO2 capture and utilization with CaO-alone for high purity syngas production ceae57100ecb7c4b2883e29079a8985d 0000-0002-7741-9278 Yuanting Qiao Yuanting Qiao true false 2024-07-15 EAAS Carbon capture and utilization (CCU) represent a promising strategy to reduce CO2 emissions and promote a sustainable economy. We report an integrated CCU (ICCU) process by integrating CO2 capture with reverse water gas shift reaction by applying simple and low-cost CaO as both sorbent and catalyst. By switching the feeding gas from CO2 source to H2 isothermally, up to 75% of captured CO2 was 100% converted into CO at 600-700 °C and the cycle performance of CaO was significantly improved under ICCU condition. In addition, the simulation confirms the significant economic advantage compared to similar traditional processes. The work could dramatically reduce the cost of materials and simplify CCU processes to advance the development and deployment of carbon neutrality technologies.One-Sentence Summary: A low-cost and widely used material, CaO, was used to not only adsorb CO2 efficiently but also in situ convert CO2 into valuable syngas with > 75% CO2 conversion to realise carbon neutrality, which is a vital target for sustainable future development. Journal Article Carbon Capture Science & Technology 1 100001 Elsevier BV 2772-6568 1 12 2021 2021-12-01 10.1016/j.ccst.2021.100001 COLLEGE NANME Engineering and Applied Sciences School COLLEGE CODE EAAS Swansea University China Scholarship Council grant 201906450023 Marie Skłodowska-Curie grant No 823745 2024-08-30T12:31:43.3001482 2024-07-15T11:14:04.3273634 Faculty of Science and Engineering School of Engineering and Applied Sciences - Chemical Engineering Shuzhuang Sun 1 Zongze Lv 2 Yuanting Qiao 0000-0002-7741-9278 3 Changlei Qin 0000-0001-6744-4608 4 Shaojun Xu 0000-0002-8026-8714 5 Chunfei Wu 0000-0001-7961-1186 6 67100__31184__9122651c24674c82a415fa0db0d812b0.pdf 67100.VoR.pdf 2024-08-30T12:29:58.2904816 Output 1549226 application/pdf Version of Record true © 2021 The Author(s). This is an open access article under the CC BY-NC-ND license. true eng http://creativecommons.org/licenses/by-nc-nd/4.0/ |
title |
Integrated CO2 capture and utilization with CaO-alone for high purity syngas production |
spellingShingle |
Integrated CO2 capture and utilization with CaO-alone for high purity syngas production Yuanting Qiao |
title_short |
Integrated CO2 capture and utilization with CaO-alone for high purity syngas production |
title_full |
Integrated CO2 capture and utilization with CaO-alone for high purity syngas production |
title_fullStr |
Integrated CO2 capture and utilization with CaO-alone for high purity syngas production |
title_full_unstemmed |
Integrated CO2 capture and utilization with CaO-alone for high purity syngas production |
title_sort |
Integrated CO2 capture and utilization with CaO-alone for high purity syngas production |
author_id_str_mv |
ceae57100ecb7c4b2883e29079a8985d |
author_id_fullname_str_mv |
ceae57100ecb7c4b2883e29079a8985d_***_Yuanting Qiao |
author |
Yuanting Qiao |
author2 |
Shuzhuang Sun Zongze Lv Yuanting Qiao Changlei Qin Shaojun Xu Chunfei Wu |
format |
Journal article |
container_title |
Carbon Capture Science & Technology |
container_volume |
1 |
container_start_page |
100001 |
publishDate |
2021 |
institution |
Swansea University |
issn |
2772-6568 |
doi_str_mv |
10.1016/j.ccst.2021.100001 |
publisher |
Elsevier BV |
college_str |
Faculty of Science and Engineering |
hierarchytype |
|
hierarchy_top_id |
facultyofscienceandengineering |
hierarchy_top_title |
Faculty of Science and Engineering |
hierarchy_parent_id |
facultyofscienceandengineering |
hierarchy_parent_title |
Faculty of Science and Engineering |
department_str |
School of Engineering and Applied Sciences - Chemical Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Chemical Engineering |
document_store_str |
1 |
active_str |
0 |
description |
Carbon capture and utilization (CCU) represent a promising strategy to reduce CO2 emissions and promote a sustainable economy. We report an integrated CCU (ICCU) process by integrating CO2 capture with reverse water gas shift reaction by applying simple and low-cost CaO as both sorbent and catalyst. By switching the feeding gas from CO2 source to H2 isothermally, up to 75% of captured CO2 was 100% converted into CO at 600-700 °C and the cycle performance of CaO was significantly improved under ICCU condition. In addition, the simulation confirms the significant economic advantage compared to similar traditional processes. The work could dramatically reduce the cost of materials and simplify CCU processes to advance the development and deployment of carbon neutrality technologies.One-Sentence Summary: A low-cost and widely used material, CaO, was used to not only adsorb CO2 efficiently but also in situ convert CO2 into valuable syngas with > 75% CO2 conversion to realise carbon neutrality, which is a vital target for sustainable future development. |
published_date |
2021-12-01T12:31:42Z |
_version_ |
1808811952573513728 |
score |
11.0241995 |