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Core–shell nanostructures for better thermoelectrics
Materials Advances, Volume: 3, Issue: 1, Pages: 125 - 141
Swansea University Authors: Rafiq Mulla, Charlie Dunnill
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DOI (Published version): 10.1039/d1ma00955a
Abstract
Substantial attempts have been made in recent decades to enhance the thermoelectric performance and find new materials. The inherent complexity and strong correlation between the electronic and thermal parameters of the materials pose serious challenges to enhance their thermoelectric performance. R...
Published in: | Materials Advances |
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ISSN: | 2633-5409 |
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Royal Society of Chemistry (RSC)
2021
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URI: | https://cronfa.swan.ac.uk/Record/cronfa59181 |
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2022-01-14T18:45:32.2525929 v2 59181 2022-01-14 Core–shell nanostructures for better thermoelectrics 1a1c32917f31df48a473a4f846068035 Rafiq Mulla Rafiq Mulla true false 0c4af8958eda0d2e914a5edc3210cd9e 0000-0003-4052-6931 Charlie Dunnill Charlie Dunnill true false 2022-01-14 CHEG Substantial attempts have been made in recent decades to enhance the thermoelectric performance and find new materials. The inherent complexity and strong correlation between the electronic and thermal parameters of the materials pose serious challenges to enhance their thermoelectric performance. Recent studies on “core–shell” nanostructures and their nanocomposites have indicated that the new strategy of creating such structurally engineered materials can help in several ways to achieve high thermoelectric performances by breaking the strongly coupled electronic and thermal parameters. Furthermore, the dependence of the Seebeck coefficient and electrical conductivity on the carrier concentrations can be altered through the core–shell structure induced energy filtering effects. This review focuses on the experimental evidence and theoretical predictions in the context of core–shell nanostructures and their composite thermoelectric materials. It also highlights the fabrication processes and concepts used to produce these novel core–shell nanostructures. Journal Article Materials Advances 3 1 125 141 Royal Society of Chemistry (RSC) 2633-5409 25 11 2021 2021-11-25 10.1039/d1ma00955a COLLEGE NANME Chemical Engineering COLLEGE CODE CHEG Swansea University European Regional Development Fund Grant: 81435 2022-01-14T18:45:32.2525929 2022-01-14T18:35:04.1716992 Faculty of Science and Engineering School of Engineering and Applied Sciences - Chemical Engineering Rafiq Mulla 1 Charlie Dunnill 0000-0003-4052-6931 2 59181__22146__108a9043005d4c9d85c9e511f2453ab3.pdf 59181.pdf 2022-01-14T18:41:28.7988012 Output 8646567 application/pdf Version of Record true This article is licensed under a Creative Commons Attribution 3.0 Unported Licence true eng http://creativecommons.org/licenses/by/3.0/ |
title |
Core–shell nanostructures for better thermoelectrics |
spellingShingle |
Core–shell nanostructures for better thermoelectrics Rafiq Mulla Charlie Dunnill |
title_short |
Core–shell nanostructures for better thermoelectrics |
title_full |
Core–shell nanostructures for better thermoelectrics |
title_fullStr |
Core–shell nanostructures for better thermoelectrics |
title_full_unstemmed |
Core–shell nanostructures for better thermoelectrics |
title_sort |
Core–shell nanostructures for better thermoelectrics |
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1a1c32917f31df48a473a4f846068035 0c4af8958eda0d2e914a5edc3210cd9e |
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1a1c32917f31df48a473a4f846068035_***_Rafiq Mulla 0c4af8958eda0d2e914a5edc3210cd9e_***_Charlie Dunnill |
author |
Rafiq Mulla Charlie Dunnill |
author2 |
Rafiq Mulla Charlie Dunnill |
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Materials Advances |
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10.1039/d1ma00955a |
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Royal Society of Chemistry (RSC) |
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description |
Substantial attempts have been made in recent decades to enhance the thermoelectric performance and find new materials. The inherent complexity and strong correlation between the electronic and thermal parameters of the materials pose serious challenges to enhance their thermoelectric performance. Recent studies on “core–shell” nanostructures and their nanocomposites have indicated that the new strategy of creating such structurally engineered materials can help in several ways to achieve high thermoelectric performances by breaking the strongly coupled electronic and thermal parameters. Furthermore, the dependence of the Seebeck coefficient and electrical conductivity on the carrier concentrations can be altered through the core–shell structure induced energy filtering effects. This review focuses on the experimental evidence and theoretical predictions in the context of core–shell nanostructures and their composite thermoelectric materials. It also highlights the fabrication processes and concepts used to produce these novel core–shell nanostructures. |
published_date |
2021-11-25T04:16:17Z |
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1763754091580751872 |
score |
11.035655 |