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Wide‐Gap Perovskites for Indoor Photovoltaics

Gregory Burwell Orcid Logo, Stefan Zeiske, Pietro Caprioglio Orcid Logo, Oskar Sandberg Orcid Logo, Austin Kay, Michael D. Farrar, Yong Kim, Henry J. Snaith Orcid Logo, Paul Meredith Orcid Logo, Ardalan Armin

Solar RRL, Volume: 8, Issue: 11

Swansea University Authors: Gregory Burwell Orcid Logo, Stefan Zeiske, Oskar Sandberg Orcid Logo, Austin Kay, Yong Kim, Paul Meredith Orcid Logo, Ardalan Armin

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DOI (Published version): 10.1002/solr.202400180

Abstract

Organic–inorganic halide perovskite semiconductors have revolutionized next-generation photovoltaics (PV) due to several characteristics such as solution-processability, gap tunability, and excellent charge generation and transport properties. This has made them very adaptable for various applicatio...

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Published in: Solar RRL
ISSN: 2367-198X 2367-198X
Published: Wiley 2024
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URI: https://cronfa.swan.ac.uk/Record/cronfa66571
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This has made them very adaptable for various applications in light harvesting and photodetection. One such rapidly growing application is indoor photovoltaics (IPV) which have the potential to power standalone Internet of Things devices. IPV requires wider optimal bandgaps than solar cells (1.8 vs 1.3 eV) due to the differences between the spectra of artificial lights versus solar radiation. For IPV applications, the active layer wide-gap perovskite must be developed systemically considering all other components of the device, such as interlayers, electrodes, and scaling. This perspective provides an overview of the potential and challenges facing perovskite-based IPV from a theoretical, material, and experimental perspective. Furthermore, accurate characterization of perovskite IPVs under simulated indoor conditions is discussed and candidate perovskite PV (PPV) systems are presented to provide insight into IPV development. These include IPV-optimized formamidinium cesium-based perovskite, wide-gap p-i-n devices, and 2D perovskite devices, tested under spectrophotometrically calibrated LED illumination at various indoor-relevant illuminances and benchmarked against thermodynamic predictions. 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spelling v2 66571 2024-06-03 Wide‐Gap Perovskites for Indoor Photovoltaics 49890fbfbe127d4ae94bc10dc2b24199 0000-0002-2534-9626 Gregory Burwell Gregory Burwell true false 0c9c5b89df9ac882c3e09dd1a9f28fc5 Stefan Zeiske Stefan Zeiske true false 9e91512a54d5aee66cd77851a96ba747 0000-0003-3778-8746 Oskar Sandberg Oskar Sandberg true false 0d9126cbd038113f697c252762b4f053 Austin Kay Austin Kay true false 512fd36e6c36e8ae0fd6f89851eee891 Yong Kim Yong Kim true false 31e8fe57fa180d418afd48c3af280c2e 0000-0002-9049-7414 Paul Meredith Paul Meredith true false 22b270622d739d81e131bec7a819e2fd Ardalan Armin Ardalan Armin true false 2024-06-03 BGPS Organic–inorganic halide perovskite semiconductors have revolutionized next-generation photovoltaics (PV) due to several characteristics such as solution-processability, gap tunability, and excellent charge generation and transport properties. This has made them very adaptable for various applications in light harvesting and photodetection. One such rapidly growing application is indoor photovoltaics (IPV) which have the potential to power standalone Internet of Things devices. IPV requires wider optimal bandgaps than solar cells (1.8 vs 1.3 eV) due to the differences between the spectra of artificial lights versus solar radiation. For IPV applications, the active layer wide-gap perovskite must be developed systemically considering all other components of the device, such as interlayers, electrodes, and scaling. This perspective provides an overview of the potential and challenges facing perovskite-based IPV from a theoretical, material, and experimental perspective. Furthermore, accurate characterization of perovskite IPVs under simulated indoor conditions is discussed and candidate perovskite PV (PPV) systems are presented to provide insight into IPV development. These include IPV-optimized formamidinium cesium-based perovskite, wide-gap p-i-n devices, and 2D perovskite devices, tested under spectrophotometrically calibrated LED illumination at various indoor-relevant illuminances and benchmarked against thermodynamic predictions. Finally, strategies required to create stable, optimized PPV devices for indoor applications are discussed. Journal Article Solar RRL 8 11 Wiley 2367-198X 2367-198X ambient photovoltaics; indoor photovoltaics; perovskite photovoltaics; testing 1 6 2024 2024-06-01 10.1002/solr.202400180 COLLEGE NANME Biosciences Geography and Physics School COLLEGE CODE BGPS Swansea University SU Library paid the OA fee (TA Institutional Deal) Engineering and Physical Sciences Research Council. Grant Number: EP/T028513/1; UK Research and Innovation. Grant Number: Research Partnership Investment Fund 2024-07-03T15:53:55.8835490 2024-06-03T11:49:16.5079150 Faculty of Science and Engineering School of Biosciences, Geography and Physics - Physics Gregory Burwell 0000-0002-2534-9626 1 Stefan Zeiske 2 Pietro Caprioglio 0000-0002-3465-2475 3 Oskar Sandberg 0000-0003-3778-8746 4 Austin Kay 5 Michael D. Farrar 6 Yong Kim 7 Henry J. Snaith 0000-0001-8511-790x 8 Paul Meredith 0000-0002-9049-7414 9 Ardalan Armin 10 66571__30520__3d0800236baa4dab813c95efd02c6275.pdf 66571_VoR.pdf 2024-06-03T11:54:46.9433003 Output 1470071 application/pdf Version of Record true © 2024 The Authors. This is an open access article under the terms of the Creative Commons Attribution License. true eng http://creativecommons.org/licenses/by/4.0/
title Wide‐Gap Perovskites for Indoor Photovoltaics
spellingShingle Wide‐Gap Perovskites for Indoor Photovoltaics
Gregory Burwell
Stefan Zeiske
Oskar Sandberg
Austin Kay
Yong Kim
Paul Meredith
Ardalan Armin
title_short Wide‐Gap Perovskites for Indoor Photovoltaics
title_full Wide‐Gap Perovskites for Indoor Photovoltaics
title_fullStr Wide‐Gap Perovskites for Indoor Photovoltaics
title_full_unstemmed Wide‐Gap Perovskites for Indoor Photovoltaics
title_sort Wide‐Gap Perovskites for Indoor Photovoltaics
author_id_str_mv 49890fbfbe127d4ae94bc10dc2b24199
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author_id_fullname_str_mv 49890fbfbe127d4ae94bc10dc2b24199_***_Gregory Burwell
0c9c5b89df9ac882c3e09dd1a9f28fc5_***_Stefan Zeiske
9e91512a54d5aee66cd77851a96ba747_***_Oskar Sandberg
0d9126cbd038113f697c252762b4f053_***_Austin Kay
512fd36e6c36e8ae0fd6f89851eee891_***_Yong Kim
31e8fe57fa180d418afd48c3af280c2e_***_Paul Meredith
22b270622d739d81e131bec7a819e2fd_***_Ardalan Armin
author Gregory Burwell
Stefan Zeiske
Oskar Sandberg
Austin Kay
Yong Kim
Paul Meredith
Ardalan Armin
author2 Gregory Burwell
Stefan Zeiske
Pietro Caprioglio
Oskar Sandberg
Austin Kay
Michael D. Farrar
Yong Kim
Henry J. Snaith
Paul Meredith
Ardalan Armin
format Journal article
container_title Solar RRL
container_volume 8
container_issue 11
publishDate 2024
institution Swansea University
issn 2367-198X
2367-198X
doi_str_mv 10.1002/solr.202400180
publisher Wiley
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Biosciences, Geography and Physics - Physics{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Biosciences, Geography and Physics - Physics
document_store_str 1
active_str 0
description Organic–inorganic halide perovskite semiconductors have revolutionized next-generation photovoltaics (PV) due to several characteristics such as solution-processability, gap tunability, and excellent charge generation and transport properties. This has made them very adaptable for various applications in light harvesting and photodetection. One such rapidly growing application is indoor photovoltaics (IPV) which have the potential to power standalone Internet of Things devices. IPV requires wider optimal bandgaps than solar cells (1.8 vs 1.3 eV) due to the differences between the spectra of artificial lights versus solar radiation. For IPV applications, the active layer wide-gap perovskite must be developed systemically considering all other components of the device, such as interlayers, electrodes, and scaling. This perspective provides an overview of the potential and challenges facing perovskite-based IPV from a theoretical, material, and experimental perspective. Furthermore, accurate characterization of perovskite IPVs under simulated indoor conditions is discussed and candidate perovskite PV (PPV) systems are presented to provide insight into IPV development. These include IPV-optimized formamidinium cesium-based perovskite, wide-gap p-i-n devices, and 2D perovskite devices, tested under spectrophotometrically calibrated LED illumination at various indoor-relevant illuminances and benchmarked against thermodynamic predictions. Finally, strategies required to create stable, optimized PPV devices for indoor applications are discussed.
published_date 2024-06-01T15:53:54Z
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