Metal organic framework composites for reduction of CO2

Liu, Kuan-Guan; Bigdeli, Fahime; Panjehpour, Akram; Larimi, Mary; Morsali, Ali; Dhakshinamoorthy, Amarajothi; Garcia, Hermenegildo

doi:10.1016/j.ccr.2023.215257

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Metal organic framework composites for reduction of CO2

Kuan-Guan Liu, Fahime Bigdeli, Akram Panjehpour, Mary Larimi

, Ali Morsali, Amarajothi Dhakshinamoorthy, Hermenegildo Garcia

Coordination Chemistry Reviews, Volume: 493, Start page: 215257

Swansea University Author: Mary Larimi

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DOI (Published version): 10.1016/j.ccr.2023.215257

Abstract

Global warming due to greenhouse gases is a major current environmental threat. In today’s world those applicable technologies which convert CO2 into valuable and environmentally friendly fuels and chemicals are of great importance. Thanks to functional sites or guests embedded in the structure, met...

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Published in:	Coordination Chemistry Reviews
ISSN:	0010-8545
Published:	Elsevier BV 2023
Online Access:	Check full text
URI:	https://cronfa.swan.ac.uk/Record/cronfa67226
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Thanks to functional sites or guests embedded in the structure, metal organic frameworks (MOFs) show a superb potential for such a conversion that is even further enhanced in MOF composites. The present review discusses the use of MOF composites, with an emphasis on their constituent components, as catalysts for CO2 reduction, converting it into various value-added and environmentally friendly chemicals such as saturated and unsaturated hydrocarbons, carboxylic acids and carboxylates, and carbon monoxide. The present review covers four major approaches for CO2 reduction, including electroreduction, photoreduction, photoelectroreduction, and hydrogenation. All reports on the design and development of appropriate MOF composites to be used in the above-mentioned CO2 reductions have been considered. 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spelling	v2 67226 2024-07-30 Metal organic framework composites for reduction of CO2 db028d01b9d62d39518f147f6bb08fa5 0000-0001-5566-171X Mary Larimi Mary Larimi true false 2024-07-30 EAAS Global warming due to greenhouse gases is a major current environmental threat. In today’s world those applicable technologies which convert CO2 into valuable and environmentally friendly fuels and chemicals are of great importance. Thanks to functional sites or guests embedded in the structure, metal organic frameworks (MOFs) show a superb potential for such a conversion that is even further enhanced in MOF composites. The present review discusses the use of MOF composites, with an emphasis on their constituent components, as catalysts for CO2 reduction, converting it into various value-added and environmentally friendly chemicals such as saturated and unsaturated hydrocarbons, carboxylic acids and carboxylates, and carbon monoxide. The present review covers four major approaches for CO2 reduction, including electroreduction, photoreduction, photoelectroreduction, and hydrogenation. All reports on the design and development of appropriate MOF composites to be used in the above-mentioned CO2 reductions have been considered. Finally, the future outlook on the use of MOF composites in CO2 reduction is provided, giving some ideas for further design highly efficient MOF composites capable of converting CO2 to value-added products. Journal Article Coordination Chemistry Reviews 493 215257 Elsevier BV 0010-8545 Heterogeneous catalysis; CO2 utilization, metal-organic framework composites; Electrocatalysis; Photocatalysis; CO2 hydrogenation 15 10 2023 2023-10-15 10.1016/j.ccr.2023.215257 COLLEGE NANME Engineering and Applied Sciences School COLLEGE CODE EAAS Swansea University The authors gratefully acknowledge from Tarbiat Modares University and the support received from the Niroo Research Institute (NRI) under the contract number 99/50420/152. This work was supported by the National Natural Science Foundation of China (Grant No. 92161106), the Natural Science Foundation of Ningxia (Grant No. 2022AAC05017), and the Foundation of State Key Laboratory of Physical Chemistry of Solid Surfaces (Grant No. 202013). Financial support by the Spanish Ministry of Science and Innovation (PDI-2021-0126071-OB-CO21) and Generalitat Valenciana (Prometeo 2021-038) is gratefully acknowledged. This study forms part of the Advanced Materials programme and was supported by MCIN with funding from European Union NextGenerationEU (PRTR-C17.I1) and by Generalitat Valenciana (Graphica MFA/2022/023. The Institute is a Center of Excellence Severo Ochoa (CEX-2021-001230-S). A.D. is beneficiary of a grant María Zambrano in Universitat Politècnica de València within the framework of the grants for the retraining in the Spanish university system (Spanish Ministry of Universities, financed by the European Union, NextGeneration EU). 2024-08-22T16:40:40.6941229 2024-07-30T11:32:50.1602058 Faculty of Science and Engineering School of Engineering and Applied Sciences - Chemical Engineering Kuan-Guan Liu 1 Fahime Bigdeli 2 Akram Panjehpour 3 Mary Larimi 0000-0001-5566-171X 4 Ali Morsali 5 Amarajothi Dhakshinamoorthy 6 Hermenegildo Garcia 0000-0002-9664-493x 7 67226__31157__873f7aee094c4e6bacb7b01c8f536aba.pdf 67226.VoR.pdf 2024-08-22T16:39:08.5143367 Output 15920271 application/pdf Version of Record true © 2024 The Authors. This is an open access article under the CC BY-NC-ND license. true eng http://creativecommons.org/licenses/by-nc-nd/4.0/
title	Metal organic framework composites for reduction of CO2
spellingShingle	Metal organic framework composites for reduction of CO2 Mary Larimi
title_short	Metal organic framework composites for reduction of CO2
title_full	Metal organic framework composites for reduction of CO2
title_fullStr	Metal organic framework composites for reduction of CO2
title_full_unstemmed	Metal organic framework composites for reduction of CO2
title_sort	Metal organic framework composites for reduction of CO2
author_id_str_mv	db028d01b9d62d39518f147f6bb08fa5
author_id_fullname_str_mv	db028d01b9d62d39518f147f6bb08fa5_***_Mary Larimi
author	Mary Larimi
author2	Kuan-Guan Liu Fahime Bigdeli Akram Panjehpour Mary Larimi Ali Morsali Amarajothi Dhakshinamoorthy Hermenegildo Garcia
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container_title	Coordination Chemistry Reviews
container_volume	493
container_start_page	215257
publishDate	2023
institution	Swansea University
issn	0010-8545
doi_str_mv	10.1016/j.ccr.2023.215257
publisher	Elsevier BV
college_str	Faculty of Science and Engineering
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description	Global warming due to greenhouse gases is a major current environmental threat. In today’s world those applicable technologies which convert CO2 into valuable and environmentally friendly fuels and chemicals are of great importance. Thanks to functional sites or guests embedded in the structure, metal organic frameworks (MOFs) show a superb potential for such a conversion that is even further enhanced in MOF composites. The present review discusses the use of MOF composites, with an emphasis on their constituent components, as catalysts for CO2 reduction, converting it into various value-added and environmentally friendly chemicals such as saturated and unsaturated hydrocarbons, carboxylic acids and carboxylates, and carbon monoxide. The present review covers four major approaches for CO2 reduction, including electroreduction, photoreduction, photoelectroreduction, and hydrogenation. All reports on the design and development of appropriate MOF composites to be used in the above-mentioned CO2 reductions have been considered. Finally, the future outlook on the use of MOF composites in CO2 reduction is provided, giving some ideas for further design highly efficient MOF composites capable of converting CO2 to value-added products.
published_date	2023-10-15T16:40:39Z
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Metal organic framework composites for reduction of CO2

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